Yep. Passing the NPVIC is the primary way forward to regulate the Electoral College to respect the popular vote.
There is too much polarization and utopian-adjacent extremists in the US political system at present.
It would take some careful thought how to improve on what the founders could not anticipate, but the current system needs a check & balance on all 3 of POTUS, COTUS, and SCOTUS to replace an unfit-for-office official.
One possibility: Perhaps a 4th branch of government with appointed-for-life by sortition panel of elders who are a safety net "board of directors" whose only function is removal of a particularly unfit elected official by unanimous vote. Their only qualifications for candidacy is that they must be of unreproachable integrity, be at least 45, have no political ties, hold no other office, and have no financial conflicts of interest. A removed elected official would be replaced according to the succession plan for their role, a special election.
Another, more radical possibility: Do away with all political parties, unlimited dark money campaign financing, and populist voting of media celebrities. Instead, fill the highest elected offices by sortition of credentialed professionals for a single 2 year term. Instead of political parties, coalitions would form around positions on issues (more nuanced than parliamentary coalition governments). COTUS and POTUS would still exist, but they would be reduced to organizational administrators who don't need to pander to billionaires. While it takes away the illusion of a sacred freedom, it replaces it with the leadership of uncorrupted, educated people who aren't constantly seeking the approval of campaign donors.