Years ago.
DRAM uses a capacitor. Those capacitors essentially hit a hard limit at around 400MHz for our traditional materials a very long time ago. This means that if you need to sequentially read random locations from RAM, you can't do it faster than 400MHz. Our only answer here is better AI prefetchers and less-random memory patterns in our software (the penalty for not prefetching is so great that theoretically less efficient algorithms can suddenly become more efficient if they are simply more predictable).
As to capacitor sizes, we've been at the volume limit for quite a while. When the capacitor is discharged, we must amplify the charge. That gets harder as the charge gets weaker and there's a fundamental limit to how small you can go. Right now, each capacitor has somewhere in the range of a mere 40,000 electrons holding the charge. Going lower dramatically increases the complexity of trying to tell the signal from the noise and dealing with ever-increasing quantum effects.
Getting more capacitors closer means a smaller diameter, but keeping the same volume means making the cylinder longer. You quickly reach a point where even dramatic increases in height (something very complicated to do in silicon) give only minuscule decreases in diameter.