It's been a while, but I remember many experiments being presented in Gleick's book ( The double pendulum being a chaotic system, or the paper showing how it was impossible to predict the distance between two points in a structure after steching and folding it)
The gist being that some systems are much more sensitive than others to initial variables - and these are what we call chaotic.
For the double pendulum, for example, you try to release the pendulum from the same point, with 0 force - no matter how precise you are, there will be variability in the position, air pressure, temperature, turbulence and whatnot that will induce a small variability. This is unavoidable - but in chaotic systems, the effects are impossible to predict i.e. the pendulum always swings differently.
The pretty pictures come from what are called "strange attractors" which are all dependent on the system you are studying because they flow from the systems attributes. It's not black magic - a simple example from the book is that heat distribution can be chaotic in liquid systems like coffee cups - so it's impossible to predict the precise temperature inside any cup given it's initial state, but we all know it's cold after an hour. This is not the best explanation for this concept, I believe the last third of the book is on the subject.
Hopefully this could help out.
Edit: if you were to plot position of the pendulum for many thousands of drops, some patterns will emerge - the pendulum moves in a "finite" set of positions, because it physically can't go in some positions after some others, for example. Or it will have the same period in rising and falling in all graphs from having close to the same initial energy but not orientation.
So it'll look neat - but it doesn't necessarily mean much.