The one thing I wish TOML had added was null. Today many TOML configs still have “nullable” keys which means you need to comment them out to unset them.
https://github.com/toml-lang/toml/issues/921
https://github.com/toml-lang/toml/issues/803
https://github.com/toml-lang/toml/issues/802
https://github.com/toml-lang/toml/issues/146
https://github.com/toml-lang/toml/issues/30
Obviously there is a bit of a demand, and it certainly has valid use cases, but also has downsides.