Earlier quoted context omitted.
Or perhaps do it the other way around? Make a Let's Encrypt subdomain-blacklisting TXT record with which the parent domain could indicate that they don't want subdomain owners to be able to create their own SSL certificates. (Useful in the case of hosted web services, for example, where the parent already owns a wildcard certificate so there's no reason for the subdomain to create one)
This is already possible using CAA DNS records, which can be used to define which CAs should be permitted to issue certificates for a domain.
Do you have any information on which CA's already support this, or whether Let's Encrypt (intends to) support this?
I'm still hoping for DANE to gain traction, though. Not necessarily as a replacement for CA's; there is value in thorough, third-party validation of certificates, but not within the current ecosystem.