I think we're going to have to try stratospheric sulfur aerosols within the next decade or so. Yes, I know it doesn't solve the ocean acidification problem. I think we should be experimenting with iron fertilization for that purpose. It might not work, or the side-effects might be too severe, but the attitude of the scientific community has been to actively suppress any such research, and I think that's a serious mistake.
It is not a choice of whether we dare to modify the biosphere, or not. We are already modifying it! That genie is not going back in the bottle. We should be learning how to modify it intentionally as well as unintentionally.