For me, systemd is the best thing since sliced bread. As a programmer, I now don't need to care about dropping privileges, managing logging, daemonization (the moment I need to do the double-fork dance again, chairs will be flying, I swear), dropping into a chroot, and do half-arsed guesses "is it up and running yet?" from a convoluted mess of shell code that looks like a bunch of hair stuck down a drain for a month.…
I can/could do without timesyncd and resolved (it's easy - just use chrony e.g.) but I like udevd being now part of systemd. It would be nice to not write /etc/udev/rules.d/ and instead have a foo.udev unit type, perhaps that is in our future (we do have .device units, but it's not the same - yet? the future). In this ballpark I think it's more on each distro picking and choosing - Ubuntu for example drank the kool-aide much deeper than RHEL - RHEL for example uses chrony out of the box, not timesyncd. However udevd and logind seem to be common across all distros now, as another user commented the KillBackground=yes setting in logind is just horrible to have as a default. The whole "homed" thing makes me sad that it's even being coded, I hope nobody adopts that (I dislike it for the same reason I dislike automount); someone out there wants it though.
The ability to dynamically edit a unit (systemctl edit) and to dynamically alter the running service constraints (systemctl set-property), all PID file type needs are handled in /run (getting rid of the nasty SysV stale unexpected crash reboot pid problem which many scripts failed to handle properly). Users having the ability to use their own private init items (systemctl --user) is great - timers, socket activation, custom login units, all very well extended down into the user's control to leverage. I'm sort of 50/50 on cron vs. timers, that's more of a use case by use case decision (example: tossing a https://healthchecks.io "&& curl ..." is just a lot quicker and easier in cron, but running a dyndns script on my laptop with a timer is nicer).
Touching on systemctl edit, it's really easy now to show folks (think a DBA team who only has the fundamental ops skill) how to quickly chain their After= and Before= needs for start/stop of their (whatever) without having to go down a rabbit hole - it's simple to use, the words and design are accessible and familiar, the method by which it works is a little obtuse (it's rooted in understanding the "dot-d" sub-include design pattern). On RHEL at least it uses nano as the default editor, annoying to me but good for casual non-vim users and easy enough to override using $EDITOR.
I used SysVinit for all the same years as everyone else (Solaris to Debian to Red Hat, ops touches it all) and wrote many my fair share of complex init units to start DB2, Oracle, java appservers (anyone remember ATG Dynamo?); systemd handles natively what 75% of that work was/is (managing PID files, watching/restarting failures, implementing namespaces/cgroups, handling dependency chains, etc.); for those complex scenarios (looking at you, Tomcat) you can still just have a unit launch a very complex shellscript "like in the old days". I haven't looked in awhile, but last time I knew in RHEL7, Red Hat did exactly that with Tomcat - just had the systemd unit launch a script.
It is, however, a real bear to debug sometimes - it's far easier to "bash -x /etc/init.d/..." and figure out what in the world is going wrong than it is to debug systemd unit failures. But, the same holds true for trying to debug DBus (if you've never tried / had to, it's not fun at all without deep dbus knowledge). I would like to see the future add more ops-oriented debugging methodology - if you've every used "pcs" (the commandline tooling for Pacemaker offered by RHEL), we could really use "systemctl debug-start" type of interfaces to the commandline offer the same experience as "bash -x" days of old. There are debug settings, they're just not ergonomically dialed in for the ops user, IMHO - systemctl debug-start would save people a lot of headaches.